- Matthew McConaughey as Buster Moon
- Andrea Bocelli as Robert Moon (buster moon's brother)
- Anne Hathaway as Penny (buster moon's new best friend)
- Brave - (Anne Hathaway ft. Matthew McConaughey) - sung by Penny & Buster Moon - Version of Sara Bareilles
- When a Heart Breaks - (Matthew McConaughey ft. Anne Hathaway) - sung by Buster Moon & Penny - Version of Ben Rector
- Beautiful Boy - (Anne Hathaway) - sung by Penny - Version of Coleen McMahon
- Hard Habit to Break - (Matthew McConaughey & Andrea Bocelli) - sung by Buster Moon & Robert Moon - Version of Chicago
- What About Me? - (Matthew McConaughey, Anne Hathaway & Andrea Bocelli) - sung by Buster Moon, Penny & Robert Moon - Version of Kenny Rogers, Kim Carnes & James Ingram
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